Silicotungstic acid explained

Silicotungstic acid or tungstosilicic acid is a heteropoly acid with the chemical formula . It forms hydrates . In freshly prepared samples, n is approximately 29, but after prolonged desiccation, n = 6. It is a white solid although impure samples appear yellow. It is used as a catalyst in the chemical industry.[1]

Applications

Silicotungstic acid is used to manufacture ethyl acetate by the alkylation of acetic acid by ethylene:

It has also been commercialized for the oxidation of ethylene to acetic acid:[1]

This route is claimed as a "greener" than methanol carbonylation. The heteropoly acid is dispersed on silica gel at 20-30 wt% to maximize catalytic ability.

It has also recently been proposed as a mediator in production of hydrogen through electrolysis of water by a process that would reduce the danger of explosion while allowing efficient hydrogen production at low current densities, conducive to hydrogen production using renewable energy.[2]

Synthesis and structure

The free acid is produced by combining sodium silicate and tungsten trioxide followed treatment of the mixture with hydrochloric acid.[3] [4] The polyoxo cluster adopts a Keggin structure, with Td point group symmetry.

Hazards

Silicotungstic acid is an irritating and odorless substance.

Notes and References

  1. Misono . Makoto . 2009 . Recent progress in the practical applications of heteropolyacid and perovskite catalysts: Catalytic technology for the sustainable society . Catalysis Today . 144 . 3–4. 285–291 . 10.1016/j.cattod.2008.10.054 .
  2. Rausch . Benjamin . Symes . Mark D. . Chisholm . Greig . Cronin . Leroy . September 12, 2014 . Decoupled catalytic hydrogen evolution from a molecular metal oxide redox mediator in water splitting . . . 345 . 6202 . 1326–1330 . 10.1126/science.1257443 . 25214625. 2014Sci...345.1326R . 20572410 .
  3. Book: Inorganic Syntheses. J. A.. Dias. S. C. L.. Dias. E.. Caliman. Keggin Structure Polyoxoometalates. Keggin Structure Polyoxometalates. 36. 210-217. 2014. 10.1002/9781118744994.ch39. 9781118744994.
  4. Handbook of Preparative Inorganic Chemistry, 2nd Ed. Edited by G. Brauer, Academic Press, 1963, NY.