Sigma complex explained

In chemistry, a sigma complex or σ-complex usually refers to a family of coordination complexes where one or more ligands interact with the metal using the bonding electrons in a sigma bond. Dihydrogen complexes are examples. Transition metal silane complexes are often especially stable sigma complexes. A particularly common subset of sigma complexes are those featuring an agostic interaction where a C–H σ-bond on one of its ligands 'leans' towards and interacts with the coordinatively unsaturated metal center to form a chelate. Transition metal alkane complexes (e.g., a methane complex) that bind solely through the C–H bond are also known but structurally characterized examples are rare, as C–H σ-bonds are generally poor electron donors, and, in many cases, the weakened C–H bond cleaves completely (C–H oxidative addition) to form a complex of type M(R)(H). In some cases, even C–C bonds function as sigma ligands.[1] Sigma complexes are of great mechanistic significance, despite their frequent fragility. They represent an initial interaction between the metal center and a hydrocarbon substrate. As such, sigma complexes are generally assumed to be intermediates prior to full oxidative addition.[2]

References

  1. Brayshaw . Simon K. . Sceats . Emma L. . Green . Jennifer C. . Weller . Andrew S. . 2007-04-24 . C–C σ complexes of rhodium . Proceedings of the National Academy of Sciences . en . 104 . 17 . 6921–6926 . 10.1073/pnas.0609824104 . free . 0027-8424 . 1855424 . 17435164.
  2. Book: Kubas , Gregory J. . Kluwer. 0-306-46465-9. Metal Dihydrogen and σ-Bond Complexes: Structure, Theory, and Reactivity. 2001-08-31.