Periodinane Explained

Periodinanes also known as λ5-iodanes are organoiodine compounds with iodine in the +5 oxidation state. These compounds are described as hypervalent because the iodine center has more than 8 valence electrons.

Periodinane compounds

The λ5-iodanes such as the Dess-Martin periodinane have square pyramidal geometry with 4 heteroatoms in basal positions and one apical phenyl group.[1]

Iodoxybenzene or iodylbenzene,, is a known oxidizing agent. Dess-Martin periodinane (1983) is another powerful oxidant and an improvement of the IBX acid already in existence in 1983. The IBX acid is prepared from 2-iodobenzoic acid and potassium bromate and sulfuric acid and is insoluble in most solvents whereas the Dess-Martin reagent prepared from reaction of the IBX acid with acetic anhydride is very soluble. The oxidation mechanism ordinarily consists of a ligand exchange reaction followed by a reductive elimination.

Uses

The predominant use of periodinanes is as oxidizing reagents replacing toxic reagents based on heavy metals.[2]

See also

External links

Notes and References

  1. 10.1002/047084289X.rt157m.pub2. 1,1,1-Triacetoxy-1,1-dihydro-1,2-benziodoxol-3(1H)-one. Encyclopedia of Reagents for Organic Synthesis. 2009. Boeckman. Robert J.. George. Kelly M.. 978-0471936237.
  2. Hypervalent iodine(V) reagents in organic synthesis Uladzimir Ladziata and Viktor V. Zhdankin Arkivoc 05-1784CR pp 26-58 2006 Article