Malononitrile Explained

Malononitrile is an organic compound nitrile with the formula . It is a colorless or white solid, although aged samples appear yellow or even brown. It is a widely used building block in organic synthesis.

Preparation and reactions

It can be prepared by dehydration of cyanoacetamide.[1] This method is mainly practiced in China where environmental rules are lax. Most commonly malononitrile is produced by the gas-phase reaction of acetonitrile and cyanogen chloride:[2]

About 20,000,000 kg are produced annually (2007). Important outlets include the synthesis of thiamine, the drug triamterene and minoxidil, and the dyes disperse Yellow 90 and disperse Blue 354.[2]

Malononitrile is relatively acidic, with a pKa of 11 in water.[3] This allows it to be used in the Knoevenagel condensation, for example in the preparation of CS gas:

Malononitrile is a suitable starting material for the Gewald reaction, where the nitrile condenses with a ketone or aldehyde in the presence of elemental sulfur and a base to produce a 2-aminothiophene.[4]

External links

Notes and References

  1. 10.15227/orgsyn.025.0063. Malononitrile. 1945. Surrey. Alexander. Organic Syntheses. 25. 63–64.
  2. Book: 10.1002/14356007.a16_063.pub2. Malonic Acid and Derivatives . Ullmann's Encyclopedia of Industrial Chemistry . 2007 . Strittmatter . Harald . Hildbrand . Stefan . Pollak . Peter . 978-3527306732 .
  3. http://evans.rc.fas.harvard.edu/pdf/evans_pKa_table.pdf Evans pKa table
  4. Sabnis, R. W.. Rangnekar, D. W.. Sonawane, N. D.. 1999. 2-Aminothiophenes By The Gewald Reaction. Journal of Heterocyclic Chemistry. 36. 2. 333–345. 2007-07-18. 10.1002/jhet.5570360203 .