Lanthanum manganite explained

Lanthanum manganite is an inorganic compound with the formula LaMnO3, often abbreviated as LMO. Lanthanum manganite is formed in the perovskite structure, consisting of oxygen octahedra with a central Mn atom. The cubic perovskite structure is distorted into an orthorhombic structure by a strong Jahn–Teller distortion of the oxygen octahedra.[1]

LaMnO3 often has lanthanum vacancies as evidenced by neutron scattering. For this reason, this material is usually referred as LaMnO3+ẟ. These vacancies generate a structure with a rhombohedral unit cell in this perovskite. A temperatures below 140 K, this LaMnO3+ẟ semiconductor exhibit a ferromagnetic order.[2]

Synthesis

Lanthanum manganite can be prepared via solid-state reactions at high temperatures, using their oxides or carbonates.[3] An alternative method is to use lanthanum nitrate and manganese nitrate as raw materials. The reaction occurs at high temperature after the solvents are vaporized.[4]

Lanthanum manganite alloys

Lanthanum manganite is an electrical insulator and an A-type antiferromagnet. It is the parent compound of several important alloys, often termed rare-earth manganites or colossal magnetoresistance oxides. These families include lanthanum strontium manganite, lanthanum calcium manganite and others.

In lanthanum manganite, both the La and the Mn are in the +3 oxidation state. Substitution of some of the La atoms by divalent atoms such as Sr or Ca induces a similar amount of tetravalent Mn4+ ions. Such substitution, or doping can induce various electronic effects, which form the basis of a rich and complex electron correlation phenomena that yield diverse electronic phase diagrams in these alloys.[5]

See also

Notes and References

  1. S. Satpathy. 1996 . . Electronic Structure of the Perovskite Oxides: La1−xCaxMnO3 . 76 . 6 . 960–963 . 10.1103/PhysRevLett.76.960 . 10061595 . 1996PhRvL..76..960S . etal. 10355/9487 . free .
  2. J. Ortiz, L. Gracia, F. Cancino, U. Pal. 2020 . . Particle dispersion and lattice distortion induced magnetic behavior of La1−xSrxMnO3 perovskite nanoparticles grown by salt-assisted solid-state synthesis . 246 . 122834 . 10.1016/j.matchemphys.2020.122834 . 213205110 . etal.
  3. Bockris. John O'M.. Otagawa. Takaaki. John Bockris. Mechanism of oxygen evolution on perovskites. The Journal of Physical Chemistry. 87. 15. 1983. 2960–2971. 0022-3654. 10.1021/j100238a048.
  4. Liu. Yuxi. Dai. Hongxing. Du. Yucheng. Deng. Jiguang. Zhang. Lei. Zhao. Zhenxuan. Au. Chak Tong. Controlled preparation and high catalytic performance of three-dimensionally ordered macroporous LaMnO3 with nanovoid skeletons for the combustion of toluene. Journal of Catalysis. 287. 2012. 149–160. 0021-9517. 10.1016/j.jcat.2011.12.015.
  5. Book: Dagotto, E. . Nanoscale Phase Separation and Colossal Magnetoresistance . 14 March 2013 . Springer . 978-3-662-05244-0 .