Iron(II) bromide explained

Iron(II) bromide refers to inorganic compounds with the chemical formula FeBr2(H2O)x. The anhydrous compound (x = 0) is a yellow or brownish-colored paramagnetic solid. The tetrahydrate is also known, all being pale colored solids. They are common precursor to other iron compounds.

Structure

Like most metal halides, FeBr2 adopts a polymeric structure consisting of isolated metal centers cross-linked with halides. It crystallizes with the CdI2 structure, featuring close-packed layers of bromide ions, between which are located Fe(II) ions in octahedral holes.[1] The packing of the halides is slightly different from that for FeCl2, which adopts the CdCl2 motif. The tetrahydrates FeX2(H2O)4 (X = Cl, Br) have similar structures, with octahedral metal centers and mutually trans halides.[2]

Synthesis and reactions

FeBr2 is synthesized using a methanol solution of concentrated hydrobromic acid and iron powder. It adds the methanol solvate [Fe(MeOH)<sub>6</sub>]Br2 together with hydrogen gas. Heating the methanol complex in a vacuum gives pure FeBr2.[3]

FeBr2 reacts with two equivalents of tetraethylammonium bromide to give [(C<sub>2</sub>H<sub>5</sub>)<sub>4</sub>N]2FeBr4.[4] FeBr2 reacts with bromide and bromine to form the intensely colored, mixed-valence species [FeBr<sub>3</sub>Br<sub>9</sub>].[5]

Magnetism

FeBr2 possesses a strong metamagnetism at 4.2 K and has long been studied as a prototypical metamagnetic compound.[6] [7]

References

  1. 10.1524/ncrs.2001.216.14.544. Refinement of the crystal structure of iron dibromide, FeBr2. Zeitschrift für Kristallographie - New Crystal Structures. 216. 1–4. 2001. Haberecht. J.. Borrmann. Η.. Kniep. R.. free.
  2. 10.1016/S0020-1693(00)80756-2. X-ray Structural Studies of FeBr2·4H2O, CoBr2·4H2O, NiCl2·4H2O and CuBr2·4H2O. Cis/Trans Selectivity in Transition Metal(II) Dihalide Tetrahydrate . 1992 . Waizumi . Kenji . Masuda . Hideki . Ohtaki . Hitoshi . Inorganica Chimica Acta . 192 . 2 . 173–181 .
  3. Book: 10.1002/9780470132456.ch20. Iron(II) Halides. 99–104. 1973. 14. Winter. G.. Inorganic Syntheses. 9780470132456.
  4. N. S. Gill, F.. B. Taylor Inorganic Syntheses 1967, volume 9, page 136-142.
  5. Holleman, A. F.; Wiberg, E. "Inorganic Chemistry" Academic Press: San Diego, 2001.
  6. Wilkinson . M. K. . Cable . J. W. . Wollan . E. O. . Koehler . W. C. . Neutron Diffraction Investigations of the Magnetic Ordering in FeBr2, CoBr2, FeCl2, and CoCl2 . Physical Review . 15 January 1959 . 113 . 2 . 497–507 . 10.1103/PhysRev.113.497. 1959PhRv..113..497W .
  7. Jacobs . I. S. . Lawrence . P. E. . Metamagnetic Phase Transitions and Hysteresis in FeCl2 . Physical Review . 10 December 1967 . 164 . 2 . 866–878 . 10.1103/PhysRev.164.866. 1967PhRv..164..866J .