Diiodine tetroxide explained

Diiodine tetraoxide, I2O4, is a chemical compound of oxygen and iodine. It belongs to the class of iodine oxides, and is a mixed oxide, consisting of iodine(III) and iodine(V) oxidation states.

Synthesis

The oxide is formed by the reaction of hot concentrated sulfuric acid on iodic acid for several days.[1]

It is formed from diiodine pentoxide and iodine in concentrated sulfuric acid or iodosyl sulfate (IO)2SO4 added to water:[2]

Physical properties

Diiodine tetraoxide is a yellow, granular powder. At temperatures above 85 °C it decomposes to diiodine pentoxide and iodine:[1]

This process is even faster at 135 °C. It dissolves in hot water to form iodate and iodide.[1] Structurally, the compound is an iodyl iodite O2I-OIO (iodine(V,III) oxide)[1] with bent IVO2 units (I–O distances 1.80 and 1.85 Å; ∠OIO angle 97°) and bent IIIIO2 units (IO distances 1.93 Å, OIO angle 95.8°). Both units are linked via I—O—I bridges to form polymeric zigzag chains (I2O4)x.[1]

Diiodine tetraoxide has a monoclinic crystal structure with the space group P21/c (space group number 14). Unit cell dimensions are a = 8.483 b = 6.696 c = 8.333 Å and β = 124.69°. Unit cell volume = 389.15 Å3. Z = 4. Density is 2.57 Mg/m3[2] [3]

Reactions

Diiodine tetroxide oxidises hydrochloric acid:[4]

References

[5]

  1. Book: Holleman-Wiberg inorganic chemistry . 2001 . Academic . San Diego, Calif. London . 0123526515. 465–466.
  2. Fjellvåg . Helmer . Kjekshus . Arne . Persson . Ingmar . Figgis . Brian N. . Liaaen-Jensen . Synnøve . Balzarini . Jan . Fransson . Bengt . Ragnarsson . Ulf . Francis . George W. . The Crystal Structure of I2O4 and its Relations to Other Iodine--Oxygen-Containing Compounds. . Acta Chemica Scandinavica . 1994 . 48 . 815–822 . 10.3891/acta.chem.scand.48-0815. free .
  3. Wu . Zhongqing . Kalia . Rajiv K. . Nakano . Aiichiro . Vashishta . Priya . First-principles calculations of the structural and dynamic properties, and the equation of state of crystalline iodine oxides I2O4, I2O5, and I2O6 . The Journal of Chemical Physics . 28 May 2011 . 134 . 20 . 10.1063/1.3590278. 21639450 .
  4. Book: Advances in Inorganic Chemistry and Radiochemistry . 1 January 1963 . Academic Press . 978-0-08-057854-5 . 77-78 . en.
  5. Book: 978-1482208689 . S.4-67. CRC Handbook of Chemistry and Physics. CRC Press . 2014. William M. Haynes.