Germanium monosulfide explained

Germanium monosulfide or Germanium(II) sulfide is the chemical compound with the formula GeS. It is a chalcogenide glass and a semiconductor.[1] Germanium sulfide is described as a red-brown powder or black crystals. Germanium(II) sulfide when dry is stable in air, hydrolyzes slowly in moist air but rapidly reacts in water forming Ge(OH)2 and then GeO.[2] It is one of a few sulfides that can be sublimed under vacuum without decomposition.[3]

Preparation

First made by Winkler by reducing GeS2 with Ge. Other methods include reduction in a stream of H2 gas, or with an excess of H3PO2 followed by vacuum sublimation.

Structure

It has a layer structure similar to that of black phosphorus. The Ge-S distances range from 247 to 300 pm. Molecular GeS in the gas phase has a Ge-S bond length of 201.21 pm.

Notes and References

  1. Sutter. Eli. Zhang. Bo. Sun. Muhua. Sutter. Peter. 2019-08-27. Few-Layer to Multilayer Germanium(II) Sulfide: Synthesis, Structure, Stability, and Optoelectronics. ACS Nano. 13. 8. 9352–9362. 10.1021/acsnano.9b03986. 31305983. 1936-0851.
  2. E. G. Rochow, E. W. Abel,1973, The Chemistry of Germanium Tin and Lead, Pergamon Press,
  3. Michael Binnewies, Robert Glaum, Marcus Schmidt, Peer Schmidt, 2012, Chemical Vapor Transport Reactions, De Gruyter,