Trichlorofluoromethane Explained

Trichlorofluoromethane, also called freon-11, CFC-11, or R-11, is a chlorofluorocarbon (CFC). It is a colorless, faintly ethereal, and sweetish-smelling liquid that boils around room temperature. CFC-11 is a Class 1 ozone-depleting substance which damages Earth's protective stratospheric ozone layer.[1] Also R-11 is not flammable at ambient temperature and pressure but it can become very combustible if heated and ignited by a strong ignition source.

Historical use

Trichlorofluoromethane was first widely used as a refrigerant. Because of its high boiling point compared to most refrigerants, it can be used in systems with a low operating pressure, making the mechanical design of such systems less demanding than that of higher-pressure refrigerants R-12 or R-22.

Trichlorofluoromethane is used as a reference compound for fluorine-19 NMR studies.

Trichlorofluoromethane was formerly used in the drinking bird novelty, largely because it has a boiling point of 23.77C. The replacement, dichloromethane, boiling point 39.6C, requires a higher ambient temperature to work.

Prior to the knowledge of the ozone depletion potential of chlorine in refrigerants and other possible harmful effects on the environment, trichlorofluoromethane was sometimes used as a cleaning/rinsing agent for low-pressure systems.[2]

Production

Trichlorofluoromethane can be obtained by reacting carbon tetrachloride with hydrogen fluoride at 435 °C and 70 atm, producing a mixture of trichlorofluoromethane, tetrafluoromethane and dichlorodifluoromethane in a ratio of 77:18:5. The reaction can also be carried out in the presence of antimony(III) chloride or antimony(V) chloride:

CCl4 + HF -> CCl3F + CF4 + CCl2F2 Trichlorofluoromethane is also formed as one of the byproducts when graphite reacts with chlorine and hydrogen fluoride at 500 °C.

Sodium hexafluorosilicate under pressure at 270 °C, titanium(IV) fluoride, chlorine trifluoride, cobalt(III) fluoride, iodine pentafluoride, and bromine trifluoride are also suitable fluorinating agents for carbon tetrachloride.[3]

CCl4 + Na2SiF6 -> CCl3F + CCl2F2 + CCl3F + NaCl + SiF4

CCl4 + BrF3 -> BrF + CCl2F2 + CCl3F

Trichlorofluoromethane was included in the production moratorium in the Montreal Protocol of 1987. It is assigned an ozone depletion potential of 1.0, and U.S. production was ended on January 1, 1996.

Regulatory challenges

In 2018, the atmospheric concentration of CFC-11 was noted by researchers to be declining more slowly than expected,[4] [5] and it subsequently emerged that it remains in widespread use as a blowing agent for polyurethane foam insulation in the construction industry of China.[6] In 2021, researchers announced that emissions declined by 20,000 U.S. tons from 2018 to 2019, which mostly reversed the previous spike in emissions.[7] In 2022, the European Commission announced an updated regulation that mandates the recovery and prevention of emissions of CFC-11 blowing agents from foam insulation in demolition waste, which is still emitted at significant scale.[8]

Dangers

R11, like most chlorofluorocarbons, forms phosgene gas when exposed to a naked flame.[9]

See also

External links

Notes and References

  1. Web site: International Treaties and Cooperation about the Protection of the Stratospheric Ozone Layer . 15 July 2015 . U.S. Environmental Protection Agency . 2021-02-14.
  2. News: R-10,R-11,R-12 GASES - ملتقى التبريد والتكييف HVACafe. 2017-05-25. ملتقى التبريد والتكييف HVACafe. 2018-05-18. ar-AR. 2018-05-18. https://web.archive.org/web/20180518130157/https://hvacafe.com/r-10-r-11-r-12-gases/. dead.
  3. Banks . A.A. . Emeléus . H.J. . Haszeldine . R. N. . Kerrigan . V. . December 1948 . 443. The reaction of bromine trifluoride and iodine pentafluoride with carbon tetrachloride, tetrabromide, and tetraiodide and with tetraiodoethylene. . . 2188–2190 . 10.1039/JR9480002188.
  4. An unexpected and persistent increase in global emissions of ozone-depleting CFC-11 . Montzka SA, Dutton GS, Yu P . etal . Nature . Springer Nature . 7705 . 413–417 . 2018 . 557 . 10.1038/s41586-018-0106-2. 29769666 . 2018Natur.557..413M . 21705434 . 1983/fd5eaf00-34b1-4689-9f23-410a54182b61 . free .
  5. Web site: It seems someone is producing a banned ozone-depleting chemical again . Johnson . Scott . 5 May 2018 . Ars Technica . 18 October 2018 . Decline of CFC-11 has slowed in recent years, pointing to a renewed source.
  6. Web site: McGrath . Matt . 9 July 2018 . China 'home foam' gas key to ozone mystery . 9 July 2018 . BBC News.
  7. Web site: Chu . Jennifer . 2021-02-10 . Reductions in CFC-11 emissions put ozone recovery back on track . .
  8. Web site: 2022-05-04 . Proposal for a regulation of the european parliament and the council on substances that deplete the ozone layer . 24 November 2022 . European Commission . European Commission-DG Environment.
  9. Web site: Orr . Bryan . 4 January 2021 . False Alarms: The Legacy of Phosgene Gas . 9 May 2022 . HVAC School.