Mertansine Explained

Mertansine, also called DM1 (and in some of its forms emtansine), is a thiol-containing maytansinoid that for therapeutic purposes is attached to a monoclonal antibody through reaction of the thiol group with a linker structure to create an antibody-drug conjugate (ADC).[1]

ADCs with this design include trastuzumab emtansine, lorvotuzumab mertansine, and cantuzumab mertansine. Some are still experimental; others are in regular clinical use.

Mechanism of action

Mertansine is a tubulin inhibitor, meaning that it inhibits the assembly of microtubules by binding to tubulin (at the rhizoxin binding site).[2]

The monoclonal antibody binds specifically to a structure (usually a protein) occurring in a tumour, thus directing mertansine into this tumour. This concept is called targeted therapy.

Uses and chemistry

The following (experimental) drugs are antibody-drug conjugates (ADC) combining monoclonal antibodies with mertansine as the cytotoxic component. Mertansine is linked via 4-mercaptovaleric acid.

ADCs include:

Emtansine

DM1 can also be linked via a more complicated structure – 4-(3-mercapto-2,5-dioxo-1-pyrrolidinylmethyl)-cylohexanecarboxylic acid or SMCC –, in which case the International Nonproprietary Name of the conjugate formed contains the word emtansine. The abbreviation comes from the chemical designation "succinimidyl-trans-4-(maleimidylmethyl) cyclohexane-1-carboxylate" which is used in the primary literature[5] as well as by the World Health Organization (WHO)[6] despite the fact that the linker contains only one imide group according to the WHO.[7]

DM1 and its attachment via these linkers result from ImmunoGen Inc research.

An example is:

Notes and References

  1. Book: Zámečník, Josef . Patologie . kolektiv autorů . PRAGER PUBLISHING . 2019 . 978-80-270-6457-1 . 1 . Praha . 276 . cs . Patology . 18 – Prediktivní patologie.
  2. [National Cancer Institute]
  3. International Nonproprietary Names for Pharmaceutical Substances (INN): List 89. WHO. 2003. 188.
  4. News: ImmunoGen reports encouraging clinical data of IMGN901. 6 December 2009. The Medical News.
  5. Clinical pharmacology of trastuzumab emtansine (T-DM1): an antibody–drug conjugate in development for the treatment of HER2-positive cancer. Cancer Chemother Pharmacol. May 2012 . 69. 5. 1229–1240. 3337408. 10.1007/s00280-011-1817-3. 22271209. Girish . Sandhya . Gupta . Manish . Wang . Bei . Lu . Dan . Krop . Ian E. . Vogel . Charles L. . Burris Iii . Howard A. . Lorusso . Patricia M. . Yi . Joo-Hee . Saad . Ola . Tong . Barbara . Chu . Yu-Waye . Holden . Scott . Joshi . Amita .
  6. International Nonproprietary Names for Pharmaceutical Substances (INN): List 103. WHO. 2010. 172.
  7. International Nonproprietary Names (INN) for pharmaceutical substances: Names for radicals, groups & others. WHO. 2012. 66f.
  8. National Cancer Institute: trastuzumab-MCC-DM1 antibody-drug conjugate
  9. http://www.immunogen.com/wt/page/trastuzumab_DM1 ImmunoGen: Trastuzumab-DM1