Dysprosium(III) chloride explained

Dysprosium(III) chloride (DyCl3), also known as dysprosium trichloride, is a compound of dysprosium and chlorine. It is a white to yellow solid which rapidly absorbs water on exposure to moist air to form a hexahydrate, DyCl3·6H2O. Simple rapid heating of the hydrate causes partial hydrolysis[1] to an oxychloride, DyOCl.

Preparation and reactions

DyCl3 is often prepared by the "ammonium chloride route", starting from either Dy2O3 or the hydrated chloride DyCl3·6H2O.[2] [3] [4] These methods produce (NH4)2[DyCl<sub>5</sub>]:

10 NH4Cl + Dy2O3 → 2 (NH4)2[DyCl<sub>5</sub>] + 6 NH3 + 3 H2O

DyCl3·6H2O + 2 NH4Cl → (NH4)2[DyCl<sub>5</sub>] + 6 H2O

The pentachloride decomposes thermally according to the following equation:

(NH4)2[DyCl<sub>5</sub>] → 2 NH4Cl + DyCl3The thermolysis reaction proceeds via the intermediacy of (NH4)[Dy<sub>2</sub>Cl<sub>7</sub>].

Treating Dy2O3 with aqueous HCl produces the hydrated chloride DyCl3·6H2O, which cannot be rendered anhydrous by heating. Instead one obtains an oxychloride:[3]

DyCl3 + H2O → DyOCl + 2 HCl

Dysprosium(III) chloride is a moderately strong Lewis acid, which ranks as "hard" according to the HSAB concept. Aqueous solutions of dysprosium chloride can be used to prepare other dysprosium(III) compounds, for example dysprosium(III) fluoride:

DyCl3 + 3 NaF → DyF3 + 3 NaCl

Uses

Dysprosium(III) chloride can be used as a starting point for the preparation of other dysprosium salts. Dysprosium metal is produced when a molten mixture of DyCl3 in eutectic LiCl-KCl is electrolysed. The reduction occurs via Dy2+, at a tungsten cathode.[5]

Precautions

Dysprosium compounds are believed to be of low to moderate toxicity, although their toxicity has not been investigated in detail.

References

  1. F. T. Edelmann, P. Poremba, in: Synthetic Methods of Organometallic and Inorganic Chemistry, (W. A. Herrmann, ed.), Vol. 6, Georg Thieme Verlag, Stuttgart, 1997.
  2. Book: Meyer , G. . The Ammonium Chloride Route to Anhydrous Rare Earth Chlorides-The Example of YCl3. The Ammonium Chloride Route to Anhydrous Rare Earth Chlorides—The Example of Ycl 3. Inorganic Syntheses. 25. 1989. 146–150. 10.1002/9780470132562.ch35. 978-0-470-13256-2.
  3. Taylor. M.D.. Carter, C.P.. Preparation of anhydrous lanthanide halides, especially iodides. Journal of Inorganic and Nuclear Chemistry. 24. 4. 387–391. 10.1016/0022-1902(62)80034-7. 1962.
  4. Book: Edelmann, F. T. . Synthetic Methods of Organometallic and Inorganic Chemistry . VI . Poremba, P. . Herrmann, W. A.. 1997 . Georg Thieme Verlag . Stuttgart . 3-13-103021-6 .
  5. Y. Castrillejo, M. R. Bermejo, A. I. Barrado, R. Pardo, E. Barrado, A. M. Martinez, Electrochimica Acta, 50, 2047-2057 (2005).