Cyclopropanes Explained

Cyclopropanes are a family of organic compounds containing the cyclopropyl group. The parent is cyclopropane .

Synthesis and reactions

Most cyclopropanes are not prepared from the parent cyclopropane, which is somewhat inert.Cyclopropyl groups are often prepared by cyclization of 1,3-difunctional alkanes. An example of the former, cyclopropyl cyanide is prepared by the reaction of 4-chlorobutyronitrile with a strong base.[1] Phenylcyclopropane is produced analogously from the 1,3-dibromide.[2]

A second major route to cyclopropanes entails addition of methylene (or its substituted derivatives) to an alkene, a process called cyclopropanation.[3]

Substituted cyclopropanes undergo the reactions associated with the cyclopropyl ring or the substituents. Vinylcyclopropanes are a special case as they undergo vinylcyclopropane rearrangement.

Applications and occurrence

Cyclopropane derivatives are numerous.[4] Many biomolecules and pharmaceutical drugs feature the cyclopropane ring. Famous example is aminocyclopropane carboxylic acid, which is the precursor to ethylene, a plant hormone.[5]

The pyrethroids are the basis of many insecticides.[6] Several cyclopropane fatty acids are known.

thumb|left|122 px|1-Aminocyclopropane-1-carboxylic acid plays an important role in the biosynthesis of the plant hormone ethylene.

References

  1. Schlatter. M. J.. Organic Syntheses. Cyclopropyl Cyanide. 1943. 23. 20. 10.15227/orgsyn.023.0020.
  2. 10.15227/orgsyn.044.0030 . Cyclopropylbenzene . Organic Syntheses . 1964 . 44 . 30 .
  3. Keiji. Maruoka. Soichi. Sakane. Hisashi. Yamamoto. 10.15227/orgsyn.067.0176 . Selective Cyclopropanation of (S)-(−)-Perillyl Alcohol: 1-Hydroxymethyl-4-(1-Methylcyclopropyl)-1-Cyclohexene . Organic Syntheses . 1989 . 67 . 176 .
  4. Book: 10.1002/0470023481. The Chemistry of the Cyclopropyl Group. The Chemistry of Functional Groups. 1995. 2. 0471940747. Rappoport. Zvi.
  5. Kieber. Joseph J.. Schaller. G. Eric. 2019-07-01. Behind the Screen: How a Simple Seedling Response Helped Unravel Ethylene Signaling in Plants. The Plant Cell. 31. 7. 1402–1403. 10.1105/tpc.19.00342. 1040-4651. 6635871. 31068448.
  6. 10.1002/1521-3773(20010618)40:12<2251::AID-ANIE2251>3.0.CO;2-R. Fascinating Natural and Artificial Cyclopropane Architectures. 2001. Faust. Rüdiger. Angewandte Chemie International Edition. 40. 12. 2251–2253. 11433485.