Cobalt(II) nitrate explained

Cobalt nitrate is the inorganic compound with the formula Co(NO3)2.xH2O. It is cobalt(II)'s salt. The most common form is the hexahydrate Co(NO3)2·6H2O, which is a red-brown deliquescent salt that is soluble in water and other polar solvents.[1]

Composition and structures

As well as the anhydrous compound Co(NO3)2, several hydrates of cobalt(II) nitrate exist. These hydrates have the chemical formula Co(NO3)2·nH2O, where n = 0, 2, 4, 6.

Anhydrous cobalt(II) nitrate adopts a three-dimensional polymeric network structure, with each cobalt(II) atom approximately octahedrally coordinated by six oxygen atoms, each from a different nitrate ion. Each nitrate ion coordinates to three cobalts.[2] The dihydrate is a two-dimensional polymer, with nitrate bridges between Co(II) centres and hydrogen bonding holding the layers together.[3] The tetrahydrate consists of discrete, octahedral [(H<sub>2</sub>O)<sub>4</sub>Co(NO<sub>3</sub>)<sub>2</sub>] molecules. The hexahydrate is better described as hexaaquacobalt(II) nitrate, [Co(OH<sub>2</sub>)<sub>6</sub>][NO<sub>3</sub>]2, as it consists of discrete [Co(OH<sub>2</sub>)<sub>6</sub>]2+ and [NO<sub>3</sub>] ions.[4] Above 55 °C, the hexahydrate converts to the trihydrate and at higher temperatures to the monohydrate.[1]

Uses and reactions

It is commonly reduced to metallic high purity cobalt.[1] It can be absorbed on to various catalyst supports for use in Fischer–Tropsch catalysis.[5] It is used in the preparation of dyes and inks.[6]

Cobalt(II) nitrate is a common starting material for the preparation of coordination complexes such as cobaloximes,[7] carbonatotetraamminecobalt(III),[8] and others.[9]

Production

The hexahydrate is prepared treating metallic cobalt or one of its oxides, hydroxides, or carbonate with nitric acid:

Co + 4 HNO3 + 4 H2O → Co(H2O)6(NO3)2 + 2 NO2

CoO + 2 HNO3 + 5 H2O → Co(H2O)6(NO3)2

CoCO3 + 2 HNO3 + 5 H2O → Co(H2O)6(NO3)2 + CO2

Notes and References

  1. John Dallas Donaldson, Detmar Beyersmann, "Cobalt and Cobalt Compounds" in Ullmann's Encyclopedia of Industrial Chemistry, Wiley-VCH, Weinheim, 2005.
  2. G. A. . Tikhomirov . K. O. . Znamenkov . I. V. . Morozov . E. . Kemnitz . S. I. . Troyanov . . 2002 . 628 . 1 . 269–273 . Anhydrous Nitrates and Nitrosonium Nitratometallates of Manganese and Cobalt, M(NO3)2, NO[Mn(NO<sub>3</sub>)<sub>3</sub>], and (NO)2[Co(NO<sub>3</sub>)<sub>4</sub>]: Synthesis and Crystal Structure . 10.1002/1521-3749(200201)628:1<269::AID-ZAAC269>3.0.CO;2-P . free .
  3. 10.1524/zkri.1976.144.1-6.133. The Crystal Structure of Cobalt Nitrate Dihydrate, Co(NO3)2·2H2O . 1976 . Ribár . B. . Milinski . N. . Herak . R. . Krstanovič . I. . Djurič . S. . Zeitschrift für Kristallographie . 144 . 1–6 . 133–138 . 1976ZK....144..133R .
  4. Cryst. Struct. Commun. . P. V. . Prelesnik . F. . Gabela . B. . Ribar . I. . Krstanovic . 2 . 4 . 1973. 581–583 . Hexaaquacobalt(II) nitrate.
  5. Ernst B, Libs S, Chaumette P, Kiennemann A. Appl. Catal. A 186 (1-2): 145-168 1999
  6. Lewis, Richard J., Sr. (2002). Hawley's Condensed Chemical Dictionary (14th Edition). John Wiley & Sons. http://www.knovel.com/knovel2/Toc.jsp?BookID=704&VerticalID=0
  7. Book: 10.1002/9780470132425.ch12. Bis(Dimethylglyoximato)Cobalt Complexes: ("Cobaloximes") . Inorganic Syntheses . 1968 . Schrauzer . G. N. . 61–70. 9780470132425 .
  8. 10.1002/9780470132371.ch55. Carbonatotetramminecobalt(III) Nitrate . Inorganic Syntheses . 6. 1960 . Schlessinger . G.. 173–175 . 9780470132371 .
  9. Book: 10.1002/9780470132456.ch15. Bis(ethylenediamine)sulfito Complexes of Cobalt(III) . Inorganic Syntheses . 1973 . Hargens . Robert D. . Min . Woonza . Henney . Robert C. . Inorganic Syntheses . 77–81 . 9780470132456 .