Chlorine monofluoride explained

Chlorine monofluoride is a volatile interhalogen compound with the chemical formula ClF. It is a colourless gas at room temperature and is stable even at high temperatures. When cooled to −100 °C, ClF condenses as a pale yellow liquid. Many of its properties are intermediate between its parent halogens, Cl2 and F2.[1]

Geometry

The molecular structure in the gas phase was determined by microwave spectroscopy; the bond length is re = 1.628341(4) Å.[2]

The bond length in the crystalline ClF is 1.628(1) Å; the lengthening relative to the free molecule is due to an interaction of the type F-Br···ClMe with a distance of 2.640(1) Å. In its molecular packing it shows very short intermolecular Cl···Cl contacts of 3.070(1) Å between neighboring molecules.[3]

Reactivity

Chlorine monofluoride is a versatile fluorinating agent, converting metals and non-metals to their fluorides and releasing Cl2 in the process. For example, it converts tungsten to tungsten hexafluoride and selenium to selenium tetrafluoride:

W + 6 ClF → WF6 + 3 Cl2

Se + 4 ClF → SeF4 + 2 Cl2

FCl can also chlorofluorinate compounds, either by addition across a multiple bond or via oxidation. For example, it adds fluorine and chlorine to the carbon of carbon monoxide, yielding carbonyl chloride fluoride:

CO + ClF →

See also

External links

Notes and References

  1. Über ein neues Chlorfluorid-CIF3. Otto Ruff, E. Ascher. Zeitschrift für anorganische und allgemeine Chemie. 1928. 176. 1. 258–270. 10.1002/zaac.19281760121.
  2. Willis . Robert E. . Clark . William W. . May 1980 . Millimeter wave measurements of the rotational spectra of ClF, BrF, BrCl, ICl, and IBr . The Journal of Chemical Physics . en . 72 . 9 . 4946–4950 . 10.1063/1.439780 . 1980JChPh..72.4946W . 0021-9606.
  3. Boese . Roland . Boese . A. Daniel . Bláser . Dieter . Antipin . Michail Yu. . Ellern . Arkadi . Seppelt . Konrad . 1997-08-04 . The Surprising Crystal Packing of Chlorinefluoride . Angewandte Chemie International Edition in English . 36 . 1314 . 1489–1492 . 10.1002/anie.199714891 . 0570-0833. free .