Dicalcium phosphate explained

Dicalcium phosphate is the calcium phosphate with the formula CaHPO4 and its dihydrate. The "di" prefix in the common name arises because the formation of the HPO42– anion involves the removal of two protons from phosphoric acid, H3PO4. It is also known as dibasic calcium phosphate or calcium monohydrogen phosphate. Dicalcium phosphate is used as a food additive, it is found in some toothpastes as a polishing agent and is a biomaterial.[1] [2]

Preparation

Dibasic calcium phosphate is produced by the neutralization of calcium hydroxide with phosphoric acid, which precipitates the dihydrate as a solid. At 60 °C the anhydrous form is precipitated:

To prevent degradation that would form hydroxyapatite, sodium pyrophosphate or trimagnesium phosphate octahydrate are added when for example, dibasic calcium phosphate dihydrate is to be used as a polishing agent in toothpaste.

In a continuous process CaCl2 can be treated with (NH4)2HPO4 to form the dihydrate:A slurry of the dihydrate is then heated to around 65–70 °C to form anhydrous CaHPO4 as a crystalline precipitate, typically as flat diamondoid crystals, which are suitable for further processing.

Dibasic calcium phosphate dihydrate is formed in "brushite" calcium phosphate cements (CPC's), which have medical applications. An example of the overall setting reaction in the formation of "β-TCP/MCPM" (β-tricalcium phosphate/monocalcium phosphate) calcium phosphate cements is:[3]

Structure

Three forms of dicalcium phosphate are known:

The structure of the anhydrous and dihydrated forms have been determined by X-ray crystallography and the structure of the monohydrate was determined by electron crystallography. The dihydrate[4] (shown in table above) as well as the monohydrate[5] adopt layered structures.

Uses and occurrence

Dibasic calcium phosphate is mainly used as a dietary supplement in prepared breakfast cereals, dog treats, enriched flour, and noodle products. It is also used as a tableting agent in some pharmaceutical preparations, including some products meant to eliminate body odor. Dibasic calcium phosphate is also found in some dietary calcium supplements (e.g. Bonexcin). It is used in poultry feed. It is also used in some toothpastes as a tartar control agent.[6]

Heating dicalcium phosphate gives dicalcium diphosphate, a useful polishing agent:

In the dihydrate (brushite) form it is found in some kidney stones and in dental calculi.[7] [8]

See also

Notes and References

  1. Book: 10.1016/B978-0-444-89307-9.50008-8 . Phosphates . Phosphorus - an Outline of its Chemistry, Biochemistry and Uses . 20 . 169–305 . Studies in Inorganic Chemistry . 1995 . 9780444893079 . Corbridge . D. E. C. .
  2. 10.1039/C3RA00166K . Bioactive ceramics: From bone grafts to tissue engineering . RSC Advances . 3 . 28 . 11116 . 2013 . Salinas . Antonio J. . Vallet-Regí . María . 2013RSCAd...311116S .
  3. 10.1016/j.actbio.2011.08.005 . 21856456 . Dicalcium phosphate cements: Brushite and monetite . Acta Biomaterialia . 8 . 2 . 474–487 . 2012 . Tamimi . Faleh . Sheikh . Zeeshan . Barralet . Jake .
  4. 10.1039/J19710003725 . Crystal structure of brushite, calcium hydrogen orthophosphate dihydrate: A neutron-diffraction investigation . Journal of the Chemical Society A: Inorganic, Physical, Theoretical . 3725 . 1971 . Curry . N. A. . Jones . D. W. .
  5. Lu. Bing-Qiang. Willhammar. Tom. Sun. Ben-Ben. Hedin. Niklas. Gale. Julian D.. Gebauer. Denis. 2020-03-24. Introducing the crystalline phase of dicalcium phosphate monohydrate. Nature Communications. en. 11. 1. 1546. 10.1038/s41467-020-15333-6. 2041-1723. 7093545. 32210234. 2020NatCo..11.1546L.
  6. Book: 10.1002/14356007.a19_465.pub3 . Phosphoric Acid and Phosphates . Ullmann's Encyclopedia of Industrial Chemistry . 2008 . Schrödter . Klaus . Bettermann . Gerhard . Staffel . Thomas . Wahl . Friedrich . Klein . Thomas . Hofmann . Thomas . 978-3527306732 . 94458523 .
  7. 10.1016/S0002-9343(03)00201-8 . 12867231 . Predictive value of kidney stone composition in the detection of metabolic abnormalities . The American Journal of Medicine . 115 . 1 . 26–32 . 2003 . Pak . Charles Y.C. . Poindexter . John R. . Adams-Huet . Beverley . Pearle . Margaret S. .
  8. Book: 10.1016/B978-0-08-055294-1.00178-1 . Bioactive Ceramics: Physical Chemistry . Comprehensive Biomaterials . 187–221 . 2011 . Rey . C. . Combes . C. . Drouet . C. . Grossin . D. . 9780080552941 .