Xenon hexafluoride explained

Xenon hexafluoride is a noble gas compound with the formula XeF6. It is one of the three binary fluorides of xenon that have been studied experimentally, the other two being XeF2 and XeF4. All known are exergonic and stable at normal temperatures. XeF6 is the strongest fluorinating agent of the series. It is a colorless solid that readily sublimes into intensely yellow vapors.

Preparation

Xenon hexafluoride can be prepared by heating of XeF2 at about 300 °C under 6 MPa (60 atmospheres) of fluorine. With as catalyst, however, this reaction can proceed at 120 °C even in xenon-fluorine molar ratios as low as 1:5.[1] [2]

Structure

The structure of XeF6 required several years to establish in contrast to the cases of and . In the gas phase the compound is monomeric. VSEPR theory predicts that due to the presence of six fluoride ligands and one lone pair of electrons the structure lacks perfect octahedral symmetry, and indeed electron diffraction combined with high-level calculations indicate that the compound's point group is C3v. It is a fluxional molecule. Oh is only insignificantly higher, indicating that the minimum on the energy surface is very shallow.[3]

129Xe and 19F NMR spectroscopy indicates that in solution the compound assumes a tetrameric structure: four equivalent xenon atoms are arranged in a tetrahedron surrounded by a fluctuating array of 24 fluorine atoms that interchange positions in a "cogwheel mechanism".

Six polymorphs of are known.[4] including one that contains XeF ions with bridging F ions.[5]

Reactions

Hydrolysis

Xenon hexafluoride hydrolyzes, ultimately affording xenon trioxide:[6]

XeF6 + H2O → XeOF4 + 2 HF

XeOF4 + H2O → XeO2F2 + 2 HF

XeO2F2 + H2O → XeO3 + 2 HF

XeF6 + 3 H2O → XeO3 + 6 HF

XeF6 is a Lewis acid, binding one and two fluoride anions:

XeF6 + F → XeF

XeF + F → XeF

Octafluoroxenates

Salts of the octafluoroxenate(VI) anion

(XeF) are very stable, decomposing only above 400 °C.[7] This anion has been shown to have square antiprismatic geometry, based on single-crystal X-ray counter analysis of its nitrosonium salt, .[8] The sodium and potassium salts are formed directly from sodium fluoride and potassium fluoride:

2 NaF + →

2 KF + →

These are thermally less stable than the caesium and rubidium salts, which are synthesized by first forming the heptafluoroxenate salts:

CsF + →

RbF + →

which are then pyrolysed at 50 °C and 20 °C, respectively, to form the yellow[9] octafluoroxenate salts:[10] [11]

2 → +

2 → +

These salts are hydrolysed by water, yielding various products containing xenon and oxygen.

The two other binary fluorides of xenon do not form such stable adducts with fluoride.

With fluoride acceptors

reacts with strong fluoride acceptors such as and [12] to form the XeF cation:

+ → XeFRuF

+ → XeFAuF +

External links

Notes and References

  1. Melita Tramšek. Boris Žemva. Synthesis, Properties and Chemistry of Xenon(II) Fluoride. December 5, 2006. Acta Chim. Slov.. 53. 2. 105–116. 10.1002/chin.200721209. July 10, 2009. May 12, 2013. https://web.archive.org/web/20130512234432/http://acta.chem-soc.si/53/53-2-105.pdf. dead.
  2. Book: Xenon Hexafluoride. 10.1002/9780470132395.ch68. 9780470132395. 258–260. 2007. Chernic. C. L.. Malm. J. G.. Inorganic Syntheses. VIII.
  3. Seppelt. Konrad. June 1979. Recent Developments in the Chemistry of Some Electronegative Elements. Accounts of Chemical Research. 12. 6. 211–216. 10.1021/ar50138a004.
  4. S. . Hoyer . K. . Emmler . T. . Seppelt. The structure of xenon hexafluoride in the solid state. Journal of Fluorine Chemistry . 127 . 10. 1415–1422. 0022-1139 . 10.1016/j.jfluchem.2006.04.014 . October 2006. 2006JFluC.127.1415H .
  5. Book: Inorganic Chemistry. limited. James E. House. Academic Press. 2008. 978-0-12-356786-4. 569.
  6. Appelman . E. H. . J. G. Malm . June 1964 . Hydrolysis of Xenon Hexafluoride and the Aqueous Solution Chemistry of Xenon . Journal of the American Chemical Society . 86 . 11 . 2141–2148 . 10.1021/ja01065a009.
  7. Book: Comprehensive Inorganic Chemistry. Sulekh. Chandra. New Age International. 2004. 81-224-1512-1. 308.
  8. A.. H. . M.. Antiprismatic Coordination about Xenon: the Structure of Nitrosonium Octafluoroxenate(VI). W.. Holloway. Coyle. 173. Science. 4003. 1238–1239. 0036-8075. 10.1126/science.173.4003.1238. Williams. 17775218. Peterson. September 1971. 1971Sci...173.1238P . 22384146 .
  9. Encyclopedia: 1995. Xenon. Encyclopædia Britannica. Encyclopædia Britannica Inc..
  10. Book: Holleman. A. F.. Wiberg. E.. Inorganic Chemistry. Academic Press. San Diego. 2001. 0-12-352651-5.
  11. Book: Anorganische Chemie. limited. Erwin. Riedel. Christoph. Janiak. 7th. Walter de Gruyter. 2007. 978-3-11-018903-2. 393.
  12. Book: Advanced Inorganic Chemistry. 6th. Cotton. Wiley-India. 2007. 978-81-265-1338-3. 591.