Triptycene Explained

Triptycene is an aromatic hydrocarbon, the simplest iptycene molecule with the formula C2H2(C6H4)3. It is a white solid that is soluble in organic solvents. The compound has a paddle-wheel configuration with D3h symmetry. It is named after the medieval three-piece art panel, the triptych. Several substituted triptycenes are known. Barrelenes are structurally related. Due to the rigid framework and three-dimensional geometry, derivatives of triptycene have been well researched.[1]

Synthesis

The parent triptycene was first prepared in 1942 by a multistep method.[2] It can also be prepared in one step in 28% yield from the Diels–Alder reaction of anthracene and benzyne.[3] In this method, benzyne is generated by the reaction of magnesium and 2-bromofluorobenzene.

Derivatives and applications

The hydrocarbon framework is very rigid and triptycene derivatives such as triptycene quinones[4] are therefore incorporated in many organic compounds as a molecular scaffold for various applications, such as molecular motors[5] or ligands.

For example, a bis(diphenylphosphino) derivative was used as a phosphine ligand on nickel in a highly selective hydrocyanation reaction of butadiene.[6] The reactivity of this catalyst is attributed to the large bite angle of the bidentate ligand supported by the triptycene framework.

External links

Notes and References

  1. 10.1246/cl.2010.658. Triptycene Derivatives: Synthesis and Applications. Chemistry Letters. 39. 7. 658–667. 2010. Zhao. Liwei. Li. Zhong. Wirth. Thomas.
  2. Bartlett . Paul D. . Paul Doughty Bartlett . Ryan . M. Josephine . Cohen . Saul G. . 1942 . Triptycene (9,10-o-Benzenoanthracene) . J. Am. Chem. Soc. . 64 . 11 . 2649–2653 . 10.1021/ja01263a035 .
  3. Wittig . George . 1959 . Triptycene . Org. Synth. . 39 . 75 . 10.15227/orgsyn.039.0075 .
  4. Triptycene quinones in synthesis: preparation of triptycene bis-cyclopentenedione . Spyroudis S, Xanthopoulou N . . 2003 . 2003 . vi . 95–105 . 10.3998/ark.5550190.0004.612 . free .
  5. Kelly TR, De Silva H, Silva RA . Unidirectional rotary motion in a molecular system . Nature . 401 . 6749 . 150–152 . September 1999 . 10490021 . 10.1038/43639 . 1999Natur.401..150K . 4351615 .
  6. Bini L, Müller C, Wilting J, von Chrzanowski L, Spek AL, Vogt D . Highly selective hydrocyanation of butadiene toward 3-pentenenitrile . J. Am. Chem. Soc. . 129 . 42 . 12622–12623 . October 2007 . 17902667 . 10.1021/ja074922e . 1874/26892 . free .