Transhalogenation Explained

Transhalogenation is a substitution reaction in which the halide of a halide compound is exchanged for another halide.[1]

Finkelstein reaction

A common method is halide metathesis. An example is the conversion of alkyl chloride into alkyl fluoride:

C3H5-Cl + NaF → R-F + NaCl

This kind of reaction is called Finkelstein reaction.[2] However, it is also possible, for example, to produce phosphorus fluoride compounds by transhalogenating chlorine, bromine or iodine bound to phosphorus with a metal fluoride.[3]

Details and biological use

As a halogen source for transhalogenation, metal halides (such as sodium fluoride or lithium fluoride) are often used, but also the use of onium halides is possible. Transhalogenation has been described as a gentle method for the synthesis of fluoroorganylboranes. It is also possible to produce aryliodides from the corresponding aryl chlorides or aryl bromides.

One investigation showed a possibility to perform transhalogenation by means of genetically modified enzymes (haloalkanes dehalogenases, HLDs).

Literature

References

  1. Book: 10.1002/9780470771723.ch3. Formation of carbon-halogen bonds . Halides, Pseudo-Halides and Azides: Part 2 (1983) . 1983 . Hudlicky . Milos . Hudlicky . Tomas . 1021–1172 . 9780470771723 .
  2. Book: Yoel Sasson. PATai's Chemistry of Functional Groups. PATai's Chemistry of Functional Groups. Formation of Carbon-Halogen Bonds (Cl, Br, I). John Wiley & Sons, Ltd. Chichester, UK. pp. pat0011. 978-0-470-68253-1. 2009-12-15. 10.1002/9780470682531.pat0011.
  3. DE . 68918542T . Verfahren zur Transhalogenierung einer Halogenphosphor-Verbindung mit Fluorwasserstoff . 1989-08-30 .