Chloramine-T Explained

Chloramine-T is the organic compound with the formula CH3C6H4SO2NClNa. Both the anhydrous salt and its trihydrate are known. Both are white powders. Chloramine-T is used as a reagent in organic synthesis.[1] [2] It is commonly used as cyclizing agent in the synthesis of aziridine, oxadiazole, isoxazole and pyrazoles.[2] It's inexpensive, has low toxicity and acts as a oxidizing agent. In addition, it also acts as a source of nitrogen anions and electrophilic cations. It may undergo degradation on long term exposure to atmosphere such that care must be taken during its storage.

Reactions

Chloramine-T contains active (electrophilic) chlorine. Its reactivity is similar to that of sodium hypochlorite. Aqueous solutions of chloramine-T are slightly basic (pH typically 8.5). The pKa of the closely related N-chlorophenylsulfonamide C6H5SO2NClH is 9.5.[1]

It is prepared by oxidation of toluenesulfonamide with sodium hypochlorite, with the latter being produced in situ from sodium hydroxide and chlorine (Cl2):[1]

Uses

Reagent in amidohydroxylation

The Sharpless oxyamination converts an alkene to a vicinal aminoalcohol. A common source of the amido component of this reaction is chloramine-T.[3] Vicinal aminoalcohols are important products in organic synthesis and recurring pharmacophores in drug discovery.

Oxidant

Chloramine-T is a strong oxidant. It oxidizes hydrogen sulfide to sulfur and mustard gas to yield a harmless crystalline sulfimide.

It converts iodide to iodine monochloride (ICl). ICl rapidly undergoes electrophilic substitution predominantly with activated aromatic rings, such as those of the amino acid tyrosine. Thus, chloramine-T is used to incorporate iodine into peptides and proteins. Chloramine-T together with iodogen or lactoperoxidase is commonly used for labeling peptides and proteins with radioiodine isotopes.[4]

Certifications

External links

Notes and References

  1. 10.1021/cr60311a005. Chloramine T and Related N-halogeno-N-metallo reagents. Chemical Reviews. 78. 65–79. 1978. Campbell. Malcolm M.. Johnson. Graham..
  2. Nayak . Yogeesha N. . Gaonkar . Santosh L. . Saleh . Ebraheem Abdu Musad . Dawsari . Abdullah Mohammed A. L. . Harshitha . Husain . Kakul . Hassan . Ismail . 2022-03-01 . Chloramine-T (N-chloro-p-toluenesulfonamide sodium salt), a versatile reagent in organic synthesis and analytical chemistry: An up to date review . Journal of Saudi Chemical Society . en . 26 . 2 . 101416 . 10.1016/j.jscs.2021.101416 . 1319-6103. free .
  3. Bodkin . J. A. . McLeod . M. D. . The Sharpless asymmetric aminohydroxylation . J. Chem. Soc., Perkin Trans. 1 . 2002 . 2002 . 24 . 2733–2746 . 10.1039/b111276g.
  4. Book: Rösch, F.. Radiochemistry and Radiopharmaceutical Chemistry in Life Sciences . 4 . Kluwer Academic Publishers . Dordrecht, Boston, London .