Tetra-n-butylammonium iodide explained

Tetra-n-butylammonium iodide (TBAI) is a quaternary ammonium salt with an iodide counterion. It is used for synthesizing tetra-n-butylammonium triiodide by mixing with iodine.

Properties

The solid crystal of tetra-n-butylammonium iodide is in the monoclinic crystal system. It has space group C2/c. The unit cell has dimensions a=14.2806 b=14.1864 c=19.5951 β=111.149. There are eight formulae in the unit cell (Z=8), which has volume 3702.4 Å3.[1]

The enthalpy of formation ΔfH0 of tetra-n-butylammonium iodide is −499 kJ/mol, which is lower than that for the bromide or chloride (−540, −564 kJ/mol).[2]

At lower temperatures with water tetra-n-butylammonium iodide forms a clathrate hydrate.[2] The tetra-n-butylammonium cation is large and hydrophobic. The absolute enthalpy of hydration (from gas phase) is −260 kJ/mol.[2]

The He(I) photoelectron spectrum of tetra-n-butylammonium iodide contains a peak at 11 eV due to the tetra-n-butylammonium cation, and at 7 and 8 eV due to iodide.[3]

See also

Notes and References

  1. Prukała . Wiesław . Marciniec . Bogdan . Kubicki . Maciej . Tetra-n-butylammonium iodide: a space-group revision . Acta Crystallographica Section E . 28 February 2007 . 63 . 3 . o1464–o1466 . 10.1107/S1600536807008446. 2007AcCrE..63O1464P .
  2. Nagano . Yatsuhisa . Mizuno . Hideki . Sakiyama . Minoru . Fujiwara . Tadayuki . Kondo . Yasuhiko . Hydration enthalpy of tetra-n-butylammonium ion . The Journal of Physical Chemistry . March 1991 . 95 . 6 . 2536–2540 . 10.1021/j100159a079.
  3. Ballard . R.E. . Jones . Jimmy . Sutherland . Elizabeth . He(I) photoelectron spectrum of tetra-N-butylammonium iodide and bromide in solution. The effects of surface activity . Chemical Physics Letters . December 1984 . 112 . 4 . 310–312 . 10.1016/0009-2614(84)85747-4. 1984CPL...112..310B .