Square antiprismatic molecular geometry explained

Examples:,
Symmetry Group:D4d
Atom Direction:8
Mu:0

In chemistry, the square antiprismatic molecular geometry describes the shape of compounds where eight atoms, groups of atoms, or ligands are arranged around a central atom, defining the vertices of a square antiprism.[1] This shape has D4d symmetry and is one of the three common shapes for octacoordinate transition metal complexes, along with the dodecahedron and the bicapped trigonal prism.[2] [3]

Like with other high coordination numbers, eight-coordinate compounds are often distorted from idealized geometries, as illustrated by the structure of Na3TaF8. In this case, with the small Na+ ions, lattice forces are strong. With the diatomic cation NO+, the lattice forces are weaker, such as in (NO)2XeF8, which crystallizes with a more idealized square antiprismatic geometry.

Examples

Square prismatic geometry and cubic geometry

Square prismatic geometry (D4h) is much less common compared to the square antiprism. An example of a molecular species with square prismatic geometry (a slightly flattened cube) is octafluoroprotactinate(V), [PaF<sub>8</sub>]3–, as found in its sodium salt, Na3PaF8.[4] While local cubic 8-coordination is common in ionic lattices (e.g., Ca2+ in CaF2), and some 8-coordinate actinide complexes are approximately cubic, there are no reported examples of rigorously cubic 8-coordinate molecular species. A number of other rare geometries for 8-coordination are also known.

References

  1. Aspects of the Stereochemistry of Eight-Coordination. 179–249. D. L. Kepert. Progress in Inorganic Chemistry. 24. 10.1002/9780470166253.ch4. 1978. 9780470166253.
  2. Eight-Coordination. Jeremy K. Burdett. Roald Hoffmann. Robert C. Fay. Inorganic Chemistry. 1978. 17. 9. 2553–2568. 10.1021/ic50187a041.
  3. Wells A.F. (1984) Structural Inorganic Chemistry 5th edition Oxford Science Publications
  4. Brown . D. . Easey . J. F. . Rickard . C. E. F. . 1969 . Cubic co-ordination: crystal structure of sodium octafluoroprotactinate(V) . Journal of the Chemical Society A: Inorganic, Physical, Theoretical . en . 1161 . 10.1039/j19690001161 . 0022-4944.