Ruthenium pentacarbonyl explained

Ruthenium pentacarbonyl is the organoruthenium compound with the formula Ru(CO)5. It is a colorless, light-sensitive liquid that readily decarbonylates upon standing at room temperature. It is of academic interest as an intermediate for the synthesis of metal carbonyl complexes.

Preparation

Ru(CO)5 was originally prepared by carbonylation of ruthenium salts in the presence of a reducing agent.[1] A more recent preparation involves photolysis of triruthenium dodecacarbonyl in the presence of carbon monoxide:[2]

Ru3(CO)12 + 3 CO 3 Ru(CO)5It is characterized by two intense νCO bands in the IR spectrum at 2038 and 2003 cm−1 (hexane solution).[2]

Comparisons of M(CO)5 (M = Fe, Ru, Os)

Whereas Fe(CO)5 is completely robust at room temperature, samples of Ru(CO)5 are typically reddish owing to contamination by Ru3(CO)12. The conversion is rapid in solution. Os(CO)5 requires heating to 80 °C to effect conversion to triosmium dodecacarbonyl.[3]

References

  1. W. Manchot, Wilhelm J. Manchot "Darstellung von Rutheniumcarbonylen und -nitrosylen" Zeitschrift für Anorganische und Allgemeine Chemie 1936, volume 226, pp. 385-415.
  2. Adams, R. D.; Barnard, T. S.; Cortopassi, J. E.; Wu, W.; Li, Z. "Platinum-ruthenium carbonyl cluster complexes" Inorganic Syntheses 1998, volume 32, pp. 280-284.
  3. 10.1021/om00077a026. Properties of the Pentacarbonyls of Ruthenium and Osmium. 1983. Rushman. Paul. Van Buuren. Gilbert N.. Shiralian. Mahmoud. Pomeroy. Roland K.. Organometallics. 2. 5. 693–694.