Organic nonlinear optical materials explained

Organic materials are expected to have relatively strong nonlinear optical properties due to delocalized electrons at

\pi-\pi

* orbitals. This expectation explains extensive search for better NLO materials among organic crystals.

L-arginine maleate dihydrate

L-arginine is one of the essential amino acids widely distributed in biological substances. It forms a number of salts with organic and inorganic acids showing non-linear optical properties. L-Arginine maleate dihydrate (C6H14N4O2,C4H4O4,2H2O) is one of these L-arginine salts which is a complex of strongly basic amino acid, carboxylic acid and provides useful information in relation to molecular interaction in present-day biological systems and to prebiotic self-organisms.[1] It is also a nonlinear optical material with second harmonic generation efficiency 1.68 times that of KDP.[2] L-arginine maleate dihydrate crystals are grown from solution by solvent evaporation; they belong to the triclinic space group P1.

L-methionine L-methioninium hydrogen maleate

L-methionine L-methioninium hydrogen maleate also belongs to the amino acid family. Crystals are grown by slow evaporation of an aqueous solution containing L-methionine and maleic acid, resulting in centimeter-large crystals of a non-centrosymmetric space group.[3] They were applied for second-harmonic generation of an (wavelength 1064 nm), and SHG efficiency equal to that of KDP has been obtained.

Notes and References

  1. S.L. Miller, E.L. Orgel, "The Origins of Life on the Earth", Prentice-Hall, New Jersey, 1974.
  2. Tapati. Mallik. Tanusree. Kar. Gabriele. Bocelli. Amos. Musattib. Synthesis, crystal structure and solubility of C6H14N4O2,C4H4O4,2H2O . Science and Technology of Advanced Materials. 6. March 2005. 5. 508–512. 10.1016/j.stam.2005.01.001. free.
  3. Subramanian. Natarajan. Neelamagam Rajan. Devi. Sathiya. Dhas. Martin Britto. Dhas. Shanmuganarayanan. Athimoolam. Crystal growth and structure of L-methionine L-methioninium hydrogen maleate—a new NLO material. Science and Technology of Advanced Materials. 9. July 2008. 2. 025012. 10.1088/1468-6996/9/2/025012. 27877987. 5099744. 2008STAdM...9b5012N.