Olefin conversion technology explained

Olefin Conversion Technology, also called the Phillips Triolefin Process, is the industrial process that interconverts propylene with ethylene and 2-butenes.[1] The process is also called the ethylene to propylene (ETP) process. In ETP, ethylene is dimerized to 1-butene, which is isomerized to 2-butenes. The 2-butenes are then subjected to metathesis with ethylene.

Rhenium- and molybdenum-containing heterogeneous catalysis are used. Nowadays, only the reverse reaction is practiced, i.e., the conversion of ethylene and 2-butene to propylene:[2]

CH2=CH2 + CH3CH=CHCH3 → 2 CH2=CHCH3

The technology is founded on an olefin metathesis reaction discovered at Phillips Petroleum Company.[3] The originally described process employed catalysts molybdenum hexacarbonyl, tungsten hexacarbonyl, and molybdenum oxide supported on alumina.

References

  1. Catalysis Reviews Science and Engineering. Converting Olefins to Propene: Ethene to Propene and Olefin Cracking. Vincent . Blay. Eva . Epelde. Rubén. Miravalles. Leo Alvarado. Perea. 60. 2018. 278. 10.1080/01614940.2018.1432017.
  2. Ghashghaee. Mohammad. Heterogeneous catalysts for gas-phase conversion of ethylene to higher olefins. Rev. Chem. Eng.. 2018. 34. 595-655. 10.1515/revce-2017-0003.
  3. Banks . R. L. . Bailey . G. C. . Olefin Disproportionation. A New Catalytic Process . Industrial & Engineering Chemistry Product Research and Development . 3 . 3. 170–173 . 1964 . 10.1021/i360011a002.