Nitrosonium tetrafluoroborate explained

Nitrosonium tetrafluoroborate, also called nitrosyl tetrafluoroborate, is a chemical compound with the chemical formula NOBF4. This colourless solid is used in organic synthesis as a nitrosating agent.[1]

NOBF4 is the nitrosonium salt of fluoroboric acid, and is composed of a nitrosonium cation, [NO]+, and a tetrafluoroborate anion, [BF<sub>4</sub>].

Reactions

The dominant property of NOBF4 is the oxidizing power and electrophilic character of the nitrosonium cation. It forms colored charge transfer complexes with hexamethylbenzene and with 18-crown-6. The latter, a deep yellow species, provides a means to dissolve NOBF4 in dichloromethane.[2]

Nitrosonium tetrafluoroborate may be used to prepare metal salts of the type [M<sup>II</sup>(CH<sub>3</sub>CN)<sub>''x''</sub>][BF<sub>4</sub>]2 (M = Cr, Mn, Fe, Co, Ni, Cu). The nitrosonium cation acts as the oxidizer, itself being reduced to nitric oxide gas:[3]

M + 2NOBF4 + xCH3CN → [M(CH<sub>3</sub>CN)<sub>''x''</sub>](BF4)2 + 2NO

With ferrocene the ferrocenium tetrafluoroborate is formed.[4]

In its infrared spectrum of this salt, νNO is a strong peak at 2387 cm−1.[5]

Notes and References

  1. Web site: A15806 Nitrosonium tetrafluoroborate, 98% . Alfa Aesar website . 2010-09-04.
  2. 10.1021/ic00346a008. Redox equilibria of the nitrosonium cation and of its nonbonded complexes. 1990. Lee. K. Y.. Kuchynka. D. J.. Kochi. Jay K.. Inorganic Chemistry. 29. 21. 4196–4204.
  3. 10.1002/0471224502.ch2 . . 33 . 75–83 . 11. Homoleptic Transition Metal Acetonitrile Cations with Tetrafluoroborate or Trifluoromethanesulfonate Anions . Robert A. . Heintz . Jennifer A. . Smith . Paul S. . Szalay . Amy . Weisgerber . Kim R. . Dunbar . August 2004 . 978-0-471-46075-6.
  4. Solvent and electrolyte effects on the kinetics of ferrocenium-ferrocene self-exchange. A reevaluation . Roger M. Nielson . George E. McManis . Lance K. Safford . Michael J. Weaver . . 10.1021/j100342a086 . 1989 . 93 . 5 . 2152.
  5. 10.1039/JR9630003557 . 670. The Infrared Spectrum of the Nitrosonium Ion . 1963 . Sharp . D. W. A. . Thorley . J. . Journal of the Chemical Society (Resumed) . 3557 .