2,2-Dimethylbutane Explained

2,2-Dimethylbutane, trivially known as neohexane at William Odling's 1876 suggestion,[1] is an organic compound with formula C6H14 or (H3C-)3-C-CH2-CH3. It is therefore an alkane, indeed the most compact and branched of the hexane isomers — the only one with a quaternary carbon and a butane (C4) backbone.

Synthesis

Butlerov's student V. Goryainov originally discovered neohexane in 1872 by cross-coupling of zinc ethyl with tert-butyl iodide.[2]

2,2-Dimethylbutane can be synthesised by the hydroisomerisation of 2,3-dimethylbutane using an acid catalyst.[3]

It can also be synthesised by isomerization of n-pentane in the presence of a catalyst containing combinations of one or more of palladium, platinum, rhodium and rhenium on a matrix of zeolite, alumina, silicon dioxide or other materials. Such reactions create a mixture of final products including isopentane, n-hexane, 3-methylpentane, 2-methylpentane, 2,3-dimethylbutane and 2,2-dimethylbutane. Since the composition of the final mixture is temperature dependant the desired final component can be obtained choice of catalyst and by combinations of temperature control and distillations.[4] [5] [6]

Uses

Neohexane is used as a high-octane anti-knock additive in gasoline and in the manufacture of agricultural chemicals.[7] It is also used in a number of commercial, automobile and home maintenance products, such as adhesives, electronic contact cleaners and upholstery polish sprays.[8]

In laboratory settings, it is commonly used as a probe molecule in techniques which study the active sites of metal catalysts. Such catalysts are used in hydrogen-deuterium exchange, hydrogenolysis, and isomerization reactions. It is well suited to this purpose as 2,2-dimethylbutane contains both an isobutyl and an ethyl group.[9]

See also

Notes and References

  1. Book: Philosophical Magazine . 1876 . Taylor & Francis. . en.
  2. Book: Журнал Русского физико-химического общества . 1872 . Тип-ія Б. Демакова . ru.
  3. Web site: 2,2-dimethylbutane. National Center for Biotechnology Information. 20 July 2015. 18 July 2015.
  4. Rabo . J. A. . Pickert . P. E. . Mays . R. L. . Pentane and Hexane Isomerization . Industrial & Engineering Chemistry . American Chemical Society (ACS) . 53 . 9 . 1961 . 0019-7866 . 10.1021/ie50621a029 . 733–736.
  5. Den Hartog . A. J. . Rek . P. J. M. . Botman . M. J. P. . De Vreugd . C. . Ponec . V. . Reactions of 2,2-dimethylbutane on platinum-rhenium/alumina catalysts. Effect of sulfur and chlorine on the selectivity . Langmuir . American Chemical Society (ACS) . 4 . 5 . 1988 . 0743-7463 . 10.1021/la00083a006 . 1100–1103.
  6. Brown . Ronald . Kemball . Charles . McDougall . Gordon S. . Exchange reactions of 2,2-dimethylpentane, 2,2-dimethylbutane and 2,2-dimethylpropane over Pt/SiO2 and Rh/SiO2 . Journal of the Chemical Society, Faraday Transactions . Royal Society of Chemistry (RSC) . 91 . 7 . 1995 . 0956-5000 . 10.1039/ft9959101131 . 1131.
  7. Web site: Hazardous Substance Fact Sheet - 2,2-Dimethylbutane . New Jersey Department of Health . June 2008 . 2 July 2021.
  8. Web site: 2,2-Dimethylbutane . Consumer Products Information Database . 2021 . 2 July 2021 . en.
  9. Burch . R. . Paál . Z. . The use of 2,2-dimethylbutane (neohexane) as a probe molecule of metal catalysts . Applied Catalysis A: General . Elsevier BV . 114 . 1 . 1994 . 0926-860X . 10.1016/0926-860x(94)85106-9 . 9–33.