Manganese heptoxide explained

Manganese(VII) oxide (manganese heptoxide) is an inorganic compound with the formula Manganese heptoxide is a volatile liquid with an oily consistency. It is a highly reactive and powerful oxidizer that reacts explosively with nearly any organic compound. It was first described in 1860.[1] It is the acid anhydride of permanganic acid.

Properties

The crystalline form of this chemical compound is dark green. The liquid is green by reflected light and red by transmitted light.[2] It is soluble in carbon tetrachloride, and decomposes when in contact with water.

Structure

Its solubility properties indicate a nonpolar molecular species, which is confirmed by its structure. The molecules consist of a pair of tetrahedra that share a common vertex. The vertices are occupied by oxygen atoms and at the centers of the tetrahedra are the Mn(VII) centers. The connectivity is indicated by the formula O3Mn−O−MnO3. The terminal Mn−O distances are 1.585 Å and the bridging oxygen is 1.77 Å distant from the two Mn atoms. The Mn−O−Mn angle is 120.7°.[3]

Pyrosulfate, pyrophosphate, and dichromate adopt structures similar to that of . Probably the most similar main group species is . Focusing on comparisons within the transition metal series, and are structurally similar but the Tc−O−Tc angle is 180°. Solid is not molecular but consists of crosslinked Re centers with both tetrahedral and octahedral sites;[4] in the vapour phase it is molecular with a similar structure to Tc2O7.[5]

Synthesis and reactions

arises as a dark green oil by the addition of cold concentrated to solid .[2] The reaction initially produces permanganic acid, (structurally,), which is dehydrated by cold sulfuric acid to form its anhydride, :

can react further with sulfuric acid to give the remarkable manganyl(VII) cation, which is isoelectronic with :

decomposes near room temperature, explosively so above 55 °C. The explosion can be initiated by striking the sample or by its exposure to oxidizable organic compounds. The products are and .[6] Ozone is also produced, giving a strong smell to the substance. The ozone can spontaneously ignite a piece of paper impregnated with an alcohol solution.

Manganese heptoxide reacts with hydrogen peroxide in presence of sulfuric acid, liberating oxygen and ozone:

Notes and References

  1. Aschoff, H. Ann. Phys. Chem. Ser. 2 volume 111 (1860) page 217 and page 224.
  2. Book: H. Lux. Manganese(VII) Oxide. Handbook of Preparative Inorganic Chemistry, 2nd Ed. . G. Brauer. Academic Press. 1963. NY, NY. 1. 1459–1460.
  3. Simon, A. . Dronskowski, R. . Krebs, B. . Hettich, B. . The Crystal Structure of Mn2O7 . . 1987 . 26 . 2 . 139–140 . 10.1002/anie.198701391.
  4. Krebs, B. . Mueller, A. . Beyer, H. H. . The Crystal Structure of Rhenium(VII) Oxide . . 1969 . 8 . 3 . 436–443 . 10.1021/ic50073a006.
  5. Wells A.F. (1962) Structural Inorganic Chemistry 3d edition Oxford University Press
  6. Holleman, A. F.; Wiberg, E. "Inorganic Chemistry" Academic Press: San Diego, 2001. .