Lithium tetrafluoroborate explained

Lithium tetrafluoroborate is an inorganic compound with the formula LiBF4. It is a white crystalline powder. It has been extensively tested for use in commercial secondary batteries, an application that exploits its high solubility in nonpolar solvents.[1]

Applications

Although BF4 has high ionic mobility, solutions of its Li+ salt are less conductive than other less associated salts.[1] As an electrolyte in lithium-ion batteries, LiBF4 offers some advantages relative to the more common LiPF6. It exhibits greater thermal stability[2] and moisture tolerance.[3] For example, LiBF4 can tolerate a moisture content up to 620 ppm at room temperature whereas LiPF6 readily hydrolyzes into toxic POF3 and HF gases, often destroying the battery's electrode materials. Disadvantages of the electrolyte include a relatively low conductivity and difficulties forming a stable solid electrolyte interface with graphite electrodes.

Thermal stability

Because LiBF4 and other alkali-metal salts thermally decompose to evolve boron trifluoride, the salt is commonly used as a convenient source of the chemical at the laboratory scale:[4]

LiBF4LiF + BF3

Production

LiBF4 is a byproduct in the industrial synthesis of diborane:[5]

8 BF3 + 6 LiHB2H6 + 6 LiBF4

LiBF4 can also be synthesized from LiF and BF3 in an appropriate solvent that is resistant to fluorination by BF3 (e.g. HF, BrF3, or liquified SO2):

LiF + BF3 → LiBF4

Notes and References

  1. Xu, Kang. "Nonaqueous Liquid Electrolytes for Lithium-Based Rechargeable Batteries."Chemical Reviews 2004, volume 104, pp. 4303-418.
  2. S. Zhang . K. Xu . T. Jow . Low-temperature performance of Li-ion cells with a LiBF4-based electrolyte. Journal of Solid State Electrochemistry. 2003. 7. 3. 147–151. 10.1007/s10008-002-0300-9. 96775286 . 16 February 2014.
  3. S. S. Zhang . z K. Xu . T. R. Jow . amp . Study of LiBF4 as an Electrolyte Salt for a Li-Ion Battery. Journal of the Electrochemical Society. 2002. 149. 5. A586–A590. 10.1149/1.1466857. 2002JElS..149A.586Z . 16 February 2014.
  4. Book: Robert Brotherton . Joseph Weber . Clarence Guibert . John Little . amp . Boron Compounds . 2000 . Ullmann's Encyclopedia of Industrial Chemistry . 10 . 10.1002/14356007.a04_309 . 3527306730 .
  5. Book: Brauer, Georg. Handbook of Preparative Inorganic Chemistry Vol. 1, 2nd Ed. 1963. Academic Press. New York. 978-0121266011. 773.