Hexa(tert-butoxy)dimolybdenum(III) explained

Hexa(tert-butoxy)dimolybdenum(III) is a coordination complex of molybdenum(III). It is one of the homoleptic alkoxides of molybdenum. An orange, air-sensitive solid, the complex has attracted academic attention as the precursor to many organomolybdenum derivatives. It an example of a charge-neutral complex featuring a molybdenum to molybdenum triple bond (Mo≡Mo), arising from the coupling of a pair of d3 metal centers. It can be prepared by a salt metathesis reaction from the THF complex of molybdenum trichloride and lithium tert-butoxide:[1]

2 MoCl3(thf)3 + 6 LiOBu-t → Mo2(OBu-t)6 + 6 LiCl + 6 thfThe complex and its ditungsten (W2) analogue adopt an ethane-like geometry. The metal to metal bond distance is 222 pm in the related complex Mo2(OCH2CMe3)6.[2]

See also

References

  1. Book: 10.1002/9781118744994.ch18. Dimolybdenum and Ditungsten Hexa(Alkoxides). Inorganic Syntheses. 36. 2014. Broderick. Erin M.. Browne. Samuel C.. Johnson. Marc J. A.. 95–102. 9781118744994.
  2. 10.1021/ic50173a045. The molybdenum-molybdenum triple bond. 2. Hexakis(alkoxy)dimolybdenum compounds: Preparation, properties and structural characterization of hexakis(neopentoxy)dimolybdenum. 1977. Chisholm. Malcolm H.. Cotton. F. Albert.. Murillo. Carlos A.. Reichert. William W.. Inorganic Chemistry. 16. 7. 1801–1808.