Fucoxanthin Explained

Fucoxanthin is a xanthophyll, with formula C42H58O6. It is found as an accessory pigment in the chloroplasts of brown algae and most other heterokonts, giving them a brown or olive-green color. Fucoxanthin absorbs light primarily in the blue-green to yellow-green part of the visible spectrum, peaking at around 510-525 nm by various estimates and absorbing significantly in the range of 450 to 540 nm.

Function

Carotenoids are pigments produced by plants and algae and play a role in light harvesting as part of the photosynthesis process. Xanthophylls are a subset of carotenoids, identified by the fact that they are oxygenated either as hydroxyl groups or as epoxide bridges. This makes them more water soluble than carotenes such as beta-carotene. Fucoxanthin is a xanthophyll that contributes more than 10% of the estimated total production of carotenoids in nature.[1] It is an accessory pigment found in the chloroplasts of many brown macroalgae, such as Fucus spp., and the golden-brown unicellular microalgae, the diatoms. It absorbs blue and green light at bandwidth 450-540 nm, imparting a brownish-olive color to algae.Fucoxanthin has a highly unique structure that contains both an epoxide bond and hydroxyl groups along with an allenic bond (two adjacent carbon-carbon double bonds) and a conjugated carbonyl group (carbon-oxygen double bond) in the polyene chain. All of these features provide fucoxanthin with powerful antioxidant activity.[2]

In macroalgal plastids, fucoxanthin acts like an antenna for light harvesting and energy transfer in the photosystem light harvesting complexes.[3] In diatoms like Phaeodactylum tricornutum, fucoxanthin is protein-bound along with chlorophyll to form a light harvesting protein complex.[4] Fucoxanthin is the dominant carotenoid, responsible for up to 60% of the energy transfer to chlorophyll a in diatoms [5] When bound to protein, the absorption spectrum of fucoxanthin expands from 450-540 nm to 390-580 nm, a range that is useful in aquatic environments.[6]

Sources

Fucoxanthin is present in brown seaweeds and diatoms and was first isolated from Fucus, Dictyota, and Laminaria by Willstätter and Page in 1914.[7] Seaweeds are commonly consumed in south-east Asia and certain countries in Europe, while diatoms are single-cell planktonic microalgae characterized by a golden-brown color, due to their high content of Fucoxanthin. Generally, diatoms contain up to 4 times more Fucoxanthin than seaweed, making diatoms a viable source for fucoxanthin industrially.[8] Diatoms can be grown in controlled environments (such as photobioreactors). Brown seaweeds are mostly grown in the open sea, often exposed to metals and metalloids.[9]

Bioavailability

Limited studies of fucoxanthin in humans indicate low bioavailability.[7]

See also

Notes and References

  1. Dembitsky VM, Maoka T . Allenic and cumulenic lipids . Progress in Lipid Research . 46 . 6 . 328–75 . November 2007 . 17765976 . 10.1016/j.plipres.2007.07.001 .
  2. Hu T, Liu D, Chen Y, Wu J, Wang S . Antioxidant activity of sulfated polysaccharide fractions extracted from Undaria pinnitafida in vitro . International Journal of Biological Macromolecules . 46 . 2 . 193–8 . March 2010 . 20025899 . 10.1016/j.ijbiomac.2009.12.004 .
  3. Owens TG, Wold ER . Light-Harvesting Function in the Diatom Phaeodactylum tricornutum: I. Isolation and Characterization of Pigment-Protein Complexes . Plant Physiology . 80 . 3 . 732–8 . March 1986 . 16664694 . 1075192 . 10.1104/pp.80.3.732.
  4. Guglielmi G, Lavaud J, Rousseau B, Etienne AL, Houmard J, Ruban AV . The light-harvesting antenna of the diatom Phaeodactylum tricornutum. Evidence for a diadinoxanthin-binding subcomplex . The FEBS Journal . 272 . 17 . 4339–48 . September 2005 . 16128804 . 10.1111/j.1742-4658.2005.04846.x . free .
  5. Papagiannakis E, van Stokkum IH, Fey H, Büchel C, van Grondelle R . Spectroscopic characterization of the excitation energy transfer in the fucoxanthin-chlorophyll protein of diatoms . Photosynthesis Research . 86 . 1–2 . 241–50 . November 2005 . 16172942 . 10.1007/s11120-005-1003-8 .
  6. Premvardhan L, Sandberg DJ, Fey H, Birge RR, Büchel C, van Grondelle R . The charge-transfer properties of the S2 state of fucoxanthin in solution and in fucoxanthin chlorophyll-a/c2 protein (FCP) based on stark spectroscopy and molecular-orbital theory . The Journal of Physical Chemistry B . 112 . 37 . 11838–53 . September 2008 . 18722413 . 2844098 . 10.1021/jp802689p .
  7. Peng J, Yuan JP, Wu CF, Wang JH . Fucoxanthin, a marine carotenoid present in brown seaweeds and diatoms: metabolism and bioactivities relevant to human health . Marine Drugs . 9 . 10 . 1806–28 . 2011-10-10 . 22072997 . 3210606 . 10.3390/md9101806 . free .
  8. Wang LJ, Fan Y, Parsons RL, Hu GR, Zhang PY, Li FL . A Rapid Method for the Determination of Fucoxanthin in Diatom . Marine Drugs . 16 . 1 . 33 . January 2018 . 29361768 . 5793081 . 10.3390/md16010033 . free .
  9. Li H, Ji H, Shi C, Gao Y, Zhang Y, Xu X, Ding H, Tang L, Xing Y . Distribution of heavy metals and metalloids in bulk and particle size fractions of soils from coal-mine brownfield and implications on human health . Chemosphere . 172 . 505–515 . April 2017 . 28104559 . 10.1016/j.chemosphere.2017.01.021 .