Knoevenagel condensation explained

In organic chemistry, the Knoevenagel condensation (pronounced as /de/) reaction is a type of chemical reaction named after German chemist Emil Knoevenagel. It is a modification of the aldol condensation.[1] [2]

A Knoevenagel condensation is a nucleophilic addition of an active hydrogen compound to a carbonyl group followed by a dehydration reaction in which a molecule of water is eliminated (hence condensation). The product is often an α,β-unsaturated ketone (a conjugated enone).

In this reaction the carbonyl group is an aldehyde or a ketone. The catalyst is usually a weakly basic amine. The active hydrogen component has the form

where Z is an electron withdrawing group. Z must be powerful enough to facilitate deprotonation to the enolate ion even with a mild base. Using a strong base in this reaction would induce self-condensation of the aldehyde or ketone.

The Hantzsch pyridine synthesis, the Gewald reaction and the Feist–Benary furan synthesis all contain a Knoevenagel reaction step. The reaction also led to the discovery of CS gas.

Doebner modification

When one of the withdrawing groups on the nucleophile is a carboxylic acid, for example, with malonic acid, the condensation product can undergo a decarboxylation process in a subsequent step. In the so-called Doebner modification[4] the base is pyridine. For example, the reaction product of acrolein and malonic acid in pyridine is trans-2,4-Pentadienoic acid with one carboxylic acid group and not two.

Scope

A Knoevenagel condensation is demonstrated in the reaction of 2-methoxybenzaldehyde 1 with the thiobarbituric acid 2 in ethanol using piperidine as a base.[5] The resulting enone 3 is a charge transfer complex molecule.

center|400px|A knoevenagel condensation

The Knoevenagel condensation is a key step in the commercial production of the antimalarial drug lumefantrine (a component of Coartem):[6]

The initial reaction product is a 50:50 mixture of E and Z isomers but because both isomers equilibrate rapidly around their common hydroxyl precursor, the more stable Z-isomer can eventually be obtained.

A multicomponent reaction featuring a Knoevenagel condensation is demonstrated in this MORE synthesis with cyclohexanone, malononitrile and 3-amino-1,2,4-triazole:[7]

Weiss–Cook reaction

The Weiss–Cook reaction consists in the synthesis of cis-bicyclo[3.3.0]octane-3,7-dione employing an acetonedicarboxylic acid ester and a diacyl (1,2 ketone). The mechanism operates in the same way as the Knoevenagel condensation:[8]

See also

Notes and References

  1. Jones, G. Org. React. 1967, 15.
  2. Emil Knoevenagel. Condensation von Malonsäure mit aromatischen Aldehyden durch Ammoniak und Amine. Condensation of malonic acid with aromatic aldehydes via ammonia and amines. Berichte der deutschen chemischen Gesellschaft. 1898. 31. 3. 2596–2619. 10.1002/cber.18980310308 . Emil Knoevenagel.
  3. Book: Organic Reactions . 204–599 . The Knoevenagel Condensation . G. Jones . 2004 . 10.1002/0471264180.or015.02 . 0471264180 .
  4. O. Doebner. Ueber die der Sorbinsäure homologen, ungesättigten Säuren mit zwei Doppelbindungen. Berichte der deutschen chemischen Gesellschaft. 1902. 35. 1136–36 . 10.1002/cber.190203501187 .
  5. 1,3-Diethyl-5-(2-methoxybenzylidene)-2-thioxodihydropyrimidine-4,6(1H,5H)-dione Abdullah Mohamed Asiria, Khaled Ahmed Alamrya Abraham F. Jalboutb, Suhong Zhang Molbank 2004, M359 http://www.mdpi.net/molbank/molbank2004/m0359.htm publication.
  6. An Improved Manufacturing Process for the Antimalaria Drug Coartem. Part II Ulrich Beutler, Peter C. Fuenfschilling, and Andreas Steinkemper Org. Process Res. Dev.; 2007; 11(3) pp. 341–45; (Article)
  7. Mild and ecofriendly tandem synthesis of 1,2,4-triazolo[4,3-a]pyrimidines in aqueous medium Arkivoc 2007 (06-2251BP) Anshu Dandia, Pritima Sarawgi, Kapil Arya, and Sarita Khaturia Link
  8. 10.1016/S0040-4039(00)72784-5 . A one-step synthesis of ketonic compounds of the pentalane, [3,3,3]- and [4,3,3]-propellane series . Tetrahedron Letters . 9 . 47 . 4885 . 1968 . Weiss . U. . Edwards . J. M. .