Dimesityldioxirane Explained

Dimesityldioxirane is a substituted dioxirane with two mesityl groups attached to the dioxirane carbon. It is a colorless crystalline substance stable in its solid state around -20 °C.[1]

Structure

The molecule possesses approximately C2 symmetry and the mesityl groups are twisted by 54.2°. The bulky mesityl groups cause steric strain which is reduced by increase in R1–C–R2 angle from 117° in dioxirane to 119.2° in dimesityldioxirane. The mesityl groups also rotate about the single bond, consequently reducing steric repulsions further.[2]

Synthesis and Uses

Dimesityldioxirane was first isolated at room temperature in pure as well as in solution form in 1994.[3] It was synthesised by irradiation of its diazo derivative in trichlorofluoromethane at 183K to form, followed by oxidation. The synthesis had a yield of 50%.

It can mainly be used as an oxidizing agent but is less oxidizing than other dioxiranes due to its stability.

See also

Notes and References

  1. Kirschfeld . Andreas . Muthusamy . Sengodagounder . Sander . Wolfram . 1994-11-17 . Dimesityldioxirane—A Dioxirane Stable in the Solid State . Angewandte Chemie International Edition in English . en . 33 . 21 . 2212–2214 . 10.1002/anie.199422121 . 0570-0833.
  2. Sander . Wolfram . Schroeder . Kerstin . Muthusamy . Sengodagounder . Kirschfeld . Andreas . Kappert . Wilhelm . Boese . Roland . Kraka . Elfi . Sosa . Carlos . Cremer . Dieter . 1997-08-01 . Dimesityldioxirane . Journal of the American Chemical Society . 119 . 31 . 7265–7270 . 10.1021/ja964280n . 0002-7863.
  3. Epoxidation using dioxiranes . Loughborough University . 1996-01-01 . PhD . en . Lesley . Walton.