Carbomethoxymethylenetriphenylphosphorane Explained

Carbomethoxymethylenetriphenylphosphorane is a chemical compound used in organic syntheses. It contains a phosphorus atom bound to three phenyl groups, and doubly bound to the alpha position of methyl acetate. It undergoes a Wittig reaction.[1] It is used in the Vitamin B12 total synthesis.

Production

Carbomethoxymethylenetriphenylphosphorane can be made via a multistep reaction using bromoacetic acid, dicyclohexylcarbodiimide, and triphenylphosphine. This makes a phosphonium salt, which is converted to the final product by sodium carbonate in water.[1]

Reactions

Carbomethoxymethylenetriphenylphosphorane reacts with aldehydes to give a two carbon atom extension. The carbomethoxymethylene group replaces the oxygen of the aldehyde to give a trans- double bond.[1]

Notes and References

  1. Keck. Gary E.. Boden. Eugene P.. Mabury. Scott A.. A useful Wittig reagent for the stereoselective synthesis of trans-.alpha.,.beta.-unsaturated thiol esters. The Journal of Organic Chemistry. March 1985. 50. 5. 709–710. 10.1021/jo00205a036.