Aldol Explained

In organic chemistry, an aldol is a structure consisting of a hydroxy group (-OH) two carbons away from either an aldehyde or a ketone. The name combines the suffix 'ol' from the alcohol and the prefix depending on the carbonyl group, either 'ald' for an aldehyde, or 'ket' for a ketone, in which case it referred to as a 'ketol'. An aldol may also use the term β-hydroxy aldehyde (or β-hydroxy ketone for a ketol). The term "aldol" may refer to 3-hydroxybutanal.[1] [2]

Aldols are the product of a carbon-carbon bond-formation reaction, giving them wide applicability as a precursor for a variety of other compounds.

Synthesis and reactions

Aldols are usually synthesized from an aldol addition reaction using two aldehydes or an aldehyde and a ketone for a ketol.[1] These reactions may also be done intramolecularly to form 5 or 6 member rings or for stereoselective syntheses in the active area of asymmetric synthesis.

Aldols may also undergo a condensation reaction in which the hydroxy group is replaced by a pi bond. The final structure is a reactive α,β-unsaturated carbonyl compound, which can also be used in a variety of other reactions:

RC(O)CH2CH(OH)R' → RC(O)CH=CHR' + H2O

Applications

Aldols synthesized from two aldehydes are usually unstable, often producing secondary compounds such as diols, unsaturated aldehydes, or alcohols. Hydroxypivaldehyde is a rare example of a distillable aldol.[3] The aldol 3-hydroxybutanal is a precursor to quinaldine, which is a precursor to the dye quinoline Yellow SS.

Aldols are also used as intermediates in the synthesis of polyketide natural products and drugs such as Oseltamivir and Epothilone.[4] [5] [6]

See also

Notes and References

  1. Kohlpainter . Christian . Schulte . Markus . Falbe . Jürgen . Lappe . Peter . Weber . Jürgen . Frey . Guido D. . 15 January 2013 . Aldehydes, Aliphatic . Ullmann's Encyclopedia of Industrial Chemistry . 7 . 10.1002/14356007.a01_321.pub3 . 9783527303854 . 1 April 2023 . Wiley Online Library.
  2. Web site: PubChem . CID 21282929 . 2023-04-15 . National Center for Biotechnology Information . en.
  3. Zhang . Yanping . Mu . Hongliang . Pan . Li . Wang . Xuling . Li . Yuesheng . 21 May 2018 . Robust Bulky [P,O] Neutral Nickel Catalysts for Copolymerization of Ethylene with Polar Vinyl Monomers . ACS Catal. . 8 . 7 . 5963–5976 . 10.1021/acscatal.8b01088 . ACS Publications.
  4. Schetter . Bernd . Mahrwald . Rainer . 2006 . Modern aldol methods for the total synthesis of polyketides . Angewandte Chemie International Edition. 45 . 45 . 7506–25 . 10.1002/anie.200602780 . 17103481 .
  5. Ghosh . Arun K. . Dawson . Zachary L. . 2009 . Synthesis of Bioactive Natural Products by Asymmetric syn- and anti-Aldol Reactions . Synthesis . 2009 . 17 . 2992–3002 . 10.1055/s-0029-1216941 . 30443084 . 6233898 . Thieme.
  6. Ko . Ji S. . Keum . Ji E. . Ko . Soo Y. . 15 October 2010 . A synthesis of oseltamivir (Tamiflu) starting from D-mannitol . J Org Chem . 75 . 20 . 7006–9 . 10.1021/jo101517g . 20866058 . National Library Of Medicine.