2,2,2-Trifluoroethanol Explained

2,2,2-Trifluoroethanol is the organic compound with the formula CF3CH2OH. Also known as TFE or trifluoroethyl alcohol, this colourless, water-miscible liquid has a smell reminiscent of ethanol. Due to the electronegativity of the trifluoromethyl group, this alcohol exhibits a stronger acidic character compared to ethanol.

Synthesis

Trifluoroethanol is produced industrially by hydrogenation or the hydride reduction of derivatives of trifluoroacetic acid, such as the esters or acyl chloride.[1]

TFE can also be prepared by hydrogenolysis of compounds of generic formula CF3−CHOH−OR (where R is hydrogen or an alkyl group containing from one to eight carbon atoms), in the presence of a palladium containing catalyst deposited on activated charcoal. As a co-catalyst for this conversion tertiary aliphatic amines like triethylamine are commonly employed.

Properties

Trifluoroethanol is used as a specialized solvent in organic chemistry.[2] [3] Oxidations of sulfur compounds using hydrogen peroxide are effectively conducted in TFE.

It competitively inhibits alcohol dehydrogenase for example.[4]

TFE forms complexes with Lewis bases such as THF or pyridine through hydrogen bonding, yielding 1:1 adducts.[5] It is classified as a hard Lewis acid and its acceptor properties are discussed in the ECW model yielding EA = 2.07 and CA = 1.06.

TFE can be used in biochemical experiments to stabilize alpha helix.[6] [7] There are also stable beta sheets in TFE, suggesting that TFE stabilizes the secondary structure the sequence has a preference for.

Reactions

Oxidation of trifluoroethanol yields trifluoroacetic acid. It also serves as a source of the trifluoroethoxy group for various chemical reactions (Still-Gennari modification of HWE reaction).

2,2,2-Trifluoroethyl vinyl ether, an inhaled drug introduced clinically under the tradename Fluoromar, features a vinyl ether of trifluorethanol. This species was prepared by the reaction of trifluoroethanol with acetylene.[1]

Safety

Trifluoroethanol is classified as toxic to blood, the reproductive system, bladder, brain, upper respiratory tract and eyes.[8] Research has shown it to be a testicular toxicant in rats and dogs.[9]

See also

References

  1. Encyclopedia: Siegemund G, Schwertfeger W, Feiring A, Smart B, Behr F, Vogel H, McKusick B, Kirsch P . Fluorine Compounds, Organic. Ullmann's Encyclopedia of Industrial Chemistry. John Wiley & Sons. 2000. 10.1002/14356007.a11_349. 3527306730.
  2. Review . Bégué JP, Bonnet-Delpon D, Crousse B . Fluorinated Alcohols: A New Medium for Selective and Clean Reaction . . 2004 . 1 . 18–29 . 10.1055/s-2003-44973.
  3. Review . Shuklov IA, Dubrovina NV, Börner A . 10.1055/s-2007-983902 . Fluorinated Alcohols as Solvents, Cosolvents and Additives in Homogeneous Catalysis . . 2925–2943 . 2007 . 2007 . 19.
  4. The competitive inhibition of yeast alcohol dehydrogenase by 2,2,2-trifluoroethanol. Biochemical Education. 26. 3. 239–242. 10.1016/s0307-4412(98)00073-9. 1998. Taber RL .
  5. Sherry AD, Purcell KF . 1970. Linear enthalpy-spectral shift correlations for 2,2,2-trifluoroethanol. Journal of Physical Chemistry. 74. 19 . 3535–3543. 10.1021/j100713a017.
  6. Pereira AF, Piccoli V, Martínez L . 2022-11-01 . Trifluoroethanol direct interactions with protein backbones destabilize α-helices . Journal of Molecular Liquids . 365 . 120209 . 10.1016/j.molliq.2022.120209 . 251914912 . 0167-7322.
  7. Zhong L, Johnson WC . Environment affects amino acid preference for secondary structure . Proceedings of the National Academy of Sciences of the United States of America . 89 . 10 . 4462–4465 . May 1992 . 1584778 . 49102 . 10.1073/pnas.89.10.4462 . 1992PNAS...89.4462Z . free .
  8. Web site: Sciencelab MSDS . 2011-11-08 . https://web.archive.org/web/20160303210222/http://www.sciencelab.com/msds.php?msdsId=9925323 . 2016-03-03 . dead .
  9. http://fscimage.fishersci.com/msds/01753.htm Fischer Scientific MSDS

External links